Michel Simon
— Mephistopheles / Old Prof. Henri Faust
Gérard Philipe
— Young Henri Faust / Young-Looking Mephistopheles
Nicole Besnard
— Marguerite the Gypsy Girl
Simone Valère
— The Princess
Carlo Ninchi
— The Prince
Raymond Cordy
— Antoine the Servant
Paolo Stoppa
— Official
Tullio Carminati
— The Diplomat
Gaston Modot
— Gypsy